Band
Title
510.0 cm-1: Fe2+-O⁻ excitation of Fe2+ & O⁻ in Siderite
Type
Raman scattering
Assignments summary
Assignment Symmetry Mode Specie(s) Molecule/Atom Bond Multiplicity Degeneracy Contribution Resonance
Fe2+-O⁻ excitation ligand-to-metal charge-transfer Fe2+
O⁻
no
Characteristics summary
Peak position
(cm-1)
Center position
(cm-1)
Width
(cm-1)
Shape Asymmetry factor Peak intensity
(cm-1)
Peak intensity relative Peak strength Integrated intensity
(cm-2)
Integrated intensity relative Integrated strength Temperature
(K)
Pressure
(bar)
510 ± 2 - 69.5 ± 1.5 symmetric 0.009 vw 0.074 m 295.0 1
Label
Fe2+-O⁻ excitation
Category
electronic transition

Evaluation

Level
uncertain assignment
Evaluation
uncertain
Comments
also attributed to Fe2+ excitation by Farsang et al. 2018, with ref. to Popkow et al. 1972
# Multiplicity type Degeneracy Other band
1 no
Primary specie
Fe2+
Primary specie
O⁻

Electronic modes

Label (type)
Fe2+-O⁻ (ligand-to-metal charge-transfer)
Composition
Fe>0.95, Mg<0.05, Mn<0.04
Texture
crystal in plot

Temperature

Temperature
295.0 ± 5.0 K

Pressure

Pressure
1 bar
Laser wavelength
532.0 nm
Sample orientation mode
unoriented
Method #1
spectrum fit
Fit function
Gaussian
Overlap
isolated
Peak
510 ± 2 cm-1 (fit peak)
Evaluation
validated
Quality
B
Comments
weak decreases with Mg fraction
FWHM
69.5 ± 1.5 cm-1 (fwhm)
Shape
symmetric
Evaluation
validated
Quality
C
Comments
independent of Mg fraction
Method
baseline corrected peak intensity
Relative intensity
0.009 ± 0.002
Strength
very weak (vw)
Evaluation
validated
Quality
D
Comments
dispersed - no trend
Method
width x peak intensity
Relative intensity
0.074 ± 0.017
Strength
medium (m)
Evaluation
recommended
Quality
D
Comments
dispersed - no trend